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  1. Free, publicly-accessible full text available February 1, 2025
  2. Free, publicly-accessible full text available February 21, 2025
  3. Subangstrom resolution has long been limited to aberration-corrected electron microscopy, where it is a powerful tool for understanding the atomic structure and properties of matter. Here, we demonstrate electron ptychography in an uncorrected scanning transmission electron microscope (STEM) with deep subangstrom spatial resolution down to 0.44 angstroms, exceeding the conventional resolution of aberration-corrected tools and rivaling their highest ptychographic resolutions​. Our approach, which we demonstrate on twisted two-dimensional materials in a widely available commercial microscope, far surpasses prior ptychographic resolutions (1 to 5 angstroms) of uncorrected STEMs. We further show how geometric aberrations can create optimized, structured beams for dose-efficient electron ptychography. Our results demonstrate that expensive aberration correctors are no longer required for deep subangstrom resolution.

     
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    Free, publicly-accessible full text available February 23, 2025
  4. Strain engineering in two-dimensional (2D) materials is a powerful but difficult to control approach to tailor material properties. Across applications, there is a need for device-compatible techniques to design strain within 2D materials. This work explores how process-induced strain engineering, commonly used by the semiconductor industry to enhance transistor performance, can be used to pattern complex strain profiles in monolayer MoS2 and 2D heterostructures. A traction–separation model is identified to predict strain profiles and extract the interfacial traction coefficient of 1.3 ± 0.7 MPa/μm and the damage initiation threshold of 16 ± 5 nm. This work demonstrates the utility to (1) spatially pattern the optical band gap with a tuning rate of 91 ± 1 meV/% strain and (2) induce interlayer heterostrain in MoS2–WSe2 heterobilayers. These results provide a CMOS-compatible approach to design complex strain patterns in 2D materials with important applications in 2D heterogeneous integration into CMOS technologies, moiré engineering, and confining quantum systems. 
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    Free, publicly-accessible full text available January 24, 2025
  5. Free, publicly-accessible full text available November 1, 2024
  6. As the field of exfoliated van der Waals electronics grows to include complex heterostructures, the variety of available in-plane symmetries and geometries becomes increasingly valuable. In this work, we present an efficient chemical vapor transport synthesis of NbSe2I2 with the triclinic space group P1̅. This material contains Nb–Nb dimers and an in-plane crystallographic angle γ = 61.3°. We show that NbSe2I2 can be exfoliated down to few-layer and monolayer structures and use Raman spectroscopy to test the preservation of the crystal structure of exfoliated thin films. The crystal structure was verified by single-crystal and powder X-ray diffraction methods. Density functional theory calculations show triclinic NbSe2I2 to be a semiconductor with a band gap of around 1 eV, with similar band structure features for bulk and monolayer crystals. The physical properties of NbSe2I2 have been characterized by transport, thermal, optical, and magnetic measurements, demonstrating triclinic NbSe2I2 to be a diamagnetic semiconductor that does not exhibit any phase transformation below room temperature. 
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    Free, publicly-accessible full text available January 4, 2025
  7. Elastocapillary rolling transfer weaves soft materials to spatial structures for programmable robotic applications. 
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    Free, publicly-accessible full text available August 25, 2024
  8. Abstract

    Sterile neutrinos only interact with the standard model through the neutrino sector, and thus represent a simple dark matter (DM) candidate with many potential astrophysical and cosmological signatures. Recently, sterile neutrinos produced through self-interactions of active neutrinos have received attention as a particle candidate that can yield the entire observed DM relic abundance without violating the most stringent constraints from X-ray observations. We examine consistency of this production mechanism with the abundance of small-scale structure in the universe, as captured by the population of ultrafaint dwarf galaxies orbiting the Milky Way, and derive a lower bound on the sterile-neutrino particle mass of 37 keV. Combining these results with previous collider and X-ray limits excludes 100% sterile-neutrino DM produced by strong neutrino self-coupling, mediated by a heavy (≳1 GeV) scalar; however, data permits sterile-neutrino DM production via a light mediator.

     
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  9. Non-equilibrium photocarriers in multilayer WSe2injected by femtosecond laser pulses exhibit extraordinary nonlinear dynamics in the presence of intense THz fields. The THz absorption in optically excited WSe2rises rapidly in the low THz field regime and gradually ramps up at high intensities. The strong THz pulses drive the photocarriers into sidebands of higher mobility and release trapped charge carriers, which consequently enhance the transient conductivity of WSe2. The spectrally analyzed conductivity reveals distinctive features, indicating that the photocarriers undergo resonant interactions such as carrier-photon scattering.

     
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  10. Language understanding is essential for the navigation agent to follow instructions. We observe two kinds of issues in the instructions that can make the navigation task challenging: 1. The mentioned landmarks are not recognizable by the navigation agent due to the different vision abilities of the instructor and the modeled agent. 2. The mentioned landmarks are applicable to multiple targets, thus not distinctive for selecting the target among the candidate viewpoints. To deal with these issues, we design a translator module for the navigation agent to convert the original instructions into easy-to-follow sub-instruction representations at each step. The translator needs to focus on the recognizable and distinctive landmarks based on the agent’s visual abilities and the observed visual environment. To achieve this goal, we create a new synthetic sub-instruction dataset and design specific tasks to train the translator and the navigation agent. We evaluate our approach on Room2Room (R2R), Room4room (R4R), and Room2Room Last (R2R-Last) datasets and achieve state-of-the-art results on multiple benchmarks. 
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    Free, publicly-accessible full text available July 1, 2024